Ordered Hierarchical Nanostructured Carbon as a Highly Efficient Cathode Catalyst Support in Proton Exchange Membrane Fuel Cell
DC Field | Value | Language |
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dc.contributor.author | Fang, Baizeng | - |
dc.contributor.author | Kim, Jung Ho | - |
dc.contributor.author | Kim, Minsik | - |
dc.contributor.author | Yu, Jong-Sung | - |
dc.date.accessioned | 2021-09-08T18:54:56Z | - |
dc.date.available | 2021-09-08T18:54:56Z | - |
dc.date.created | 2021-06-10 | - |
dc.date.issued | 2009-03-10 | - |
dc.identifier.issn | 0897-4756 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/120433 | - |
dc.description.abstract | Ordered hierarchical nanostructured carbon (OHNC) has been fabricated through inverse replication of silica template and explored for the first time to support high loading of Pt nanoparticles as cathode catalyst in proton exchange membrane fuel cells (PEMFC). The superb characteristics such as ordered hierarchical nanostructure, large surface area, and mesopore volume enable the OHNC to support high loading (60 wt %) of Pt nanoparticles with uniform dispersion and small particle size. Compared to carbon black Vulcan XC-72 (VC)-supported Pt (60 wt %), the OHNC-supported one has exhibited greatly enhanced catalytic activity toward oxygen reduction reaction by ca. 53-88% and considerably improved PEMFC performance. More importantly, unlike the VC-supported Pt catalysts, the OHNC-supported Pt (40 or 60 wt %) outperforms the OHNC-supported Pt (20 wt %) even at a low catalyst loading of 0.2 mg Pt/cm(2) in the cathode, which represents a significant breakthrough in fuel cell technology because of the expectable marked reduction in fabricating cost of the supported Pt catalyst and the corresponding system weight and considerably improved fuel cell performance. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.subject | OXYGEN REDUCTION REACTION | - |
dc.subject | ELECTROCHEMICAL HYDROGEN STORAGE | - |
dc.subject | CORE/MESOPOROUS SHELL CARBON | - |
dc.subject | COLLOID-IMPRINTED CARBON | - |
dc.subject | MESOPOROUS CARBON | - |
dc.subject | ELECTROCATALYST SUPPORT | - |
dc.subject | METHANOL OXIDATION | - |
dc.subject | NANOPARTICLE CATALYSTS | - |
dc.subject | PLATINUM NANOPARTICLES | - |
dc.subject | VAPOR-DEPOSITION | - |
dc.title | Ordered Hierarchical Nanostructured Carbon as a Highly Efficient Cathode Catalyst Support in Proton Exchange Membrane Fuel Cell | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Yu, Jong-Sung | - |
dc.identifier.doi | 10.1021/cm801467y | - |
dc.identifier.scopusid | 2-s2.0-65249158979 | - |
dc.identifier.wosid | 000263891700006 | - |
dc.identifier.bibliographicCitation | CHEMISTRY OF MATERIALS, v.21, no.5, pp.789 - 796 | - |
dc.relation.isPartOf | CHEMISTRY OF MATERIALS | - |
dc.citation.title | CHEMISTRY OF MATERIALS | - |
dc.citation.volume | 21 | - |
dc.citation.number | 5 | - |
dc.citation.startPage | 789 | - |
dc.citation.endPage | 796 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.subject.keywordPlus | OXYGEN REDUCTION REACTION | - |
dc.subject.keywordPlus | ELECTROCHEMICAL HYDROGEN STORAGE | - |
dc.subject.keywordPlus | CORE/MESOPOROUS SHELL CARBON | - |
dc.subject.keywordPlus | COLLOID-IMPRINTED CARBON | - |
dc.subject.keywordPlus | MESOPOROUS CARBON | - |
dc.subject.keywordPlus | ELECTROCATALYST SUPPORT | - |
dc.subject.keywordPlus | METHANOL OXIDATION | - |
dc.subject.keywordPlus | NANOPARTICLE CATALYSTS | - |
dc.subject.keywordPlus | PLATINUM NANOPARTICLES | - |
dc.subject.keywordPlus | VAPOR-DEPOSITION | - |
dc.subject.keywordAuthor | Hierarchical Nanostructured Carbon | - |
dc.subject.keywordAuthor | Fuel Cell | - |
dc.subject.keywordAuthor | Support | - |
dc.subject.keywordAuthor | Electrode | - |
dc.subject.keywordAuthor | Cathode Catalyst | - |
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