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Morphology controlled nanocrystalline CsPbBr3 thin-film for metal halide perovskite light emitting diodes

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dc.contributor.authorKim, B.W.-
dc.contributor.authorHeo, J.H.-
dc.contributor.authorPark, J.K.-
dc.contributor.authorLee, D.S.-
dc.contributor.authorPark, H.-
dc.contributor.authorKim, S.Y.-
dc.contributor.authorKim, J.H.-
dc.contributor.authorIm, S.H.-
dc.date.accessioned2021-12-02T10:41:49Z-
dc.date.available2021-12-02T10:41:49Z-
dc.date.created2021-08-31-
dc.date.issued2021-05-25-
dc.identifier.issn1226-086X-
dc.identifier.urihttps://scholar.korea.ac.kr/handle/2021.sw.korea/128862-
dc.description.abstractMorphology and crystal grain size of inorganic CsPbBr3 metal halide perovskite (MHP) films are controllable through a diffusion-controlled anti-solvent dripping crystallization method using an anti-solvent mixture of toluene (Tol):isopropanol (IPA). The 8:2 (v:v) Tol:IPA anti-solvent enables the production of a pinhole-free CsPbBr3 MHP film with the smallest crystal grain size and the brightest photoluminescence (PL). Accordingly, the 8:2 CsPbBr3 MHP film reveals a very uniform and strong PL mapping image. As a result, the 8:2 CsPbBr3 MHP light emitting diode (LED) exhibits ∼12.8, ∼7.4, and ∼7.9 fold enhanced maximum electroluminescence (ELmax), current efficiency (CEmax), and external quantum efficiency (EQEmax) compared to the 10:0 pristine device. The optimized 8:2 MHP LED shows an ELmax of 22,298 cd/m2, CEmax of 36.65 cd/A and EQEmax of 9.64%, respectively. In addition, the 8:2 CsPbBr3 MHP LED with controlled morphology and grain size has better operating stability than the pristine device. © 2021 The Korean Society of Industrial and Engineering Chemistry-
dc.languageEnglish-
dc.language.isoen-
dc.publisherKorean Society of Industrial Engineering Chemistry-
dc.titleMorphology controlled nanocrystalline CsPbBr3 thin-film for metal halide perovskite light emitting diodes-
dc.typeArticle-
dc.contributor.affiliatedAuthorIm, S.H.-
dc.identifier.doi10.1016/j.jiec.2021.02.028-
dc.identifier.scopusid2-s2.0-85102306234-
dc.identifier.wosid000640616000012-
dc.identifier.bibliographicCitationJournal of Industrial and Engineering Chemistry, v.97, pp.417 - 425-
dc.relation.isPartOfJournal of Industrial and Engineering Chemistry-
dc.citation.titleJournal of Industrial and Engineering Chemistry-
dc.citation.volume97-
dc.citation.startPage417-
dc.citation.endPage425-
dc.type.rimsART-
dc.type.docTypeArticle-
dc.identifier.kciidART002734443-
dc.description.journalClass1-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.description.journalRegisteredClasskci-
dc.relation.journalResearchAreaChemistry-
dc.relation.journalResearchAreaEngineering-
dc.relation.journalWebOfScienceCategoryChemistry, Multidisciplinary-
dc.relation.journalWebOfScienceCategoryEngineering, Chemical-
dc.subject.keywordPlusQUANTUM DOTS-
dc.subject.keywordPlusBRIGHT-
dc.subject.keywordPlusLUMINESCENCE-
dc.subject.keywordPlusPERFORMANCE-
dc.subject.keywordAuthorAnti-solvent dripping-
dc.subject.keywordAuthorCrystallization-
dc.subject.keywordAuthorDiffusion-
dc.subject.keywordAuthorInorganic metal halide perovskite-
dc.subject.keywordAuthorLight emitting diode-
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