Fused Bithiophene Imide Dimer-Based n-Type Polymers for High-Performance Organic Electrochemical Transistors
DC Field | Value | Language |
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dc.contributor.author | Feng, Kui | - |
dc.contributor.author | Shan, Wentao | - |
dc.contributor.author | Ma, Suxiang | - |
dc.contributor.author | Wu, Ziang | - |
dc.contributor.author | Chen, Jianhua | - |
dc.contributor.author | Guo, Han | - |
dc.contributor.author | Liu, Bin | - |
dc.contributor.author | Wang, Junwei | - |
dc.contributor.author | Li, Bangbang | - |
dc.contributor.author | Woo, Han Young | - |
dc.contributor.author | Fabiano, Simone | - |
dc.contributor.author | Huang, Wei | - |
dc.contributor.author | Guo, Xugang | - |
dc.date.accessioned | 2022-02-14T19:40:40Z | - |
dc.date.available | 2022-02-14T19:40:40Z | - |
dc.date.created | 2022-02-08 | - |
dc.date.issued | 2021-11-02 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/135776 | - |
dc.description.abstract | The development of n-type organic electrochemical transistors (OECTs) lags far behind their p-type counterparts. In order to address this dilemma, we report here two new fused bithiophene imide dimer (f-BTI2)-based n-type polymers with a branched methyl end-capped glycol side chain, which exhibit good solubility, low-lying LUMO energy levels, favorable polymer chain orientation, and efficient ion transport property, thus yielding a remarkable OECT electron mobility (mu(e)) of up to approximate to 10(-2) cm(2) V-1 s(-1) and volumetric capacitance (C*) as high as 443 F cm(-3), simultaneously. As a result, the f-BTI2TEG-FT-based OECTs deliver a record-high maximum geometry-normalized transconductance of 4.60 S cm(-1) and a maximum mu C* product of 15.2 F cm(-1) V-1 s(-1). The mu C* figure of merit is more than one order of magnitude higher than that of the state-of-the-art n-type OECTs. The emergence of f-BTI2TEG-FT brings a new paradigm for developing high-performance n-type polymers for low-power OECT applications. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.subject | STRUCTURE-PROPERTY CORRELATIONS | - |
dc.subject | SEMICONDUCTORS SYNTHESIS | - |
dc.subject | DEVICE PERFORMANCE | - |
dc.subject | DESIGN | - |
dc.title | Fused Bithiophene Imide Dimer-Based n-Type Polymers for High-Performance Organic Electrochemical Transistors | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Woo, Han Young | - |
dc.identifier.doi | 10.1002/anie.202109281 | - |
dc.identifier.scopusid | 2-s2.0-85116443879 | - |
dc.identifier.wosid | 000703116100001 | - |
dc.identifier.bibliographicCitation | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.60, no.45, pp.24198 - 24205 | - |
dc.relation.isPartOf | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | - |
dc.citation.title | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | - |
dc.citation.volume | 60 | - |
dc.citation.number | 45 | - |
dc.citation.startPage | 24198 | - |
dc.citation.endPage | 24205 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.subject.keywordPlus | DESIGN | - |
dc.subject.keywordPlus | DEVICE PERFORMANCE | - |
dc.subject.keywordPlus | SEMICONDUCTORS SYNTHESIS | - |
dc.subject.keywordPlus | STRUCTURE-PROPERTY CORRELATIONS | - |
dc.subject.keywordAuthor | electron mobility | - |
dc.subject.keywordAuthor | fused bithiophene imide dimer | - |
dc.subject.keywordAuthor | n-type polymer semiconductors | - |
dc.subject.keywordAuthor | organic electrochemical transistors | - |
dc.subject.keywordAuthor | organic electronics | - |
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