Mechanically Interlocked Polymer Electrolyte with Built-In Fast Molecular Shuttles for All-Solid-State Lithium Batteries
DC Field | Value | Language |
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dc.contributor.author | Seo, Jiae | - |
dc.contributor.author | Lee, Gwang-Hee | - |
dc.contributor.author | Hur, Joon | - |
dc.contributor.author | Sung, Myeong-Chang | - |
dc.contributor.author | Seo, Ji-Hun | - |
dc.contributor.author | Kim, Dong-Wan | - |
dc.date.accessioned | 2022-02-15T21:41:58Z | - |
dc.date.available | 2022-02-15T21:41:58Z | - |
dc.date.created | 2022-02-08 | - |
dc.date.issued | 2021-11 | - |
dc.identifier.issn | 1614-6832 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/135906 | - |
dc.description.abstract | The mobility of molecular shuttles inside a mechanically interlocked polymer (MIP) can improve the ionic conductivity and electron transport capacity of a solid polymer electrolyte (SPE) and maintain a mechanically tough structure. The polyrotaxane-based MIP electrolyte with a necklace-like molecular structure exhibits high ionic conductivity (sigma = 5.93 x 10(-3) S cm(-1) at 25 degrees C and 1.44 x 10(-2) S cm(-1) at 60 degrees C), a high Li+ ion transference number (t(+) = 0.71), and high electrochemical oxidation stability (approximate to 4.7 V vs Li+/Li). When SPEs are used in Li-based batteries, a high Coulombic efficiency (>= 98.5%), an excellent rate capability, and fast charging (>= 2C) can be achieved using a "built-in molecular shuttle" design. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.subject | IONIC-CONDUCTIVITY | - |
dc.subject | TRANSPORT | - |
dc.title | Mechanically Interlocked Polymer Electrolyte with Built-In Fast Molecular Shuttles for All-Solid-State Lithium Batteries | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Seo, Ji-Hun | - |
dc.contributor.affiliatedAuthor | Kim, Dong-Wan | - |
dc.identifier.doi | 10.1002/aenm.202102583 | - |
dc.identifier.scopusid | 2-s2.0-85116839860 | - |
dc.identifier.wosid | 000705101900001 | - |
dc.identifier.bibliographicCitation | ADVANCED ENERGY MATERIALS, v.11, no.44 | - |
dc.relation.isPartOf | ADVANCED ENERGY MATERIALS | - |
dc.citation.title | ADVANCED ENERGY MATERIALS | - |
dc.citation.volume | 11 | - |
dc.citation.number | 44 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Energy & Fuels | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalResearchArea | Physics | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.relation.journalWebOfScienceCategory | Energy & Fuels | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Physics, Applied | - |
dc.relation.journalWebOfScienceCategory | Physics, Condensed Matter | - |
dc.subject.keywordPlus | IONIC-CONDUCTIVITY | - |
dc.subject.keywordPlus | TRANSPORT | - |
dc.subject.keywordAuthor | ASSLBs | - |
dc.subject.keywordAuthor | mechanically interlocked polymers | - |
dc.subject.keywordAuthor | molecular shuttles | - |
dc.subject.keywordAuthor | polyrotaxane | - |
dc.subject.keywordAuthor | solid polymer electrolytes | - |
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