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Regioselective Synthesis of Tetrasubstituted Pyrroles by 1,3-Dipolar Cycloaddition and Spontaneous Decarboxylation
- Authors
- 김용주
- Issue Date
- 1월-2009
- Publisher
- AMER CHEMICAL SOC
- Citation
- ORGANIC LETTERS, v.11, no.1, pp.17 - 20
- Indexed
- SCOPUS
- Journal Title
- ORGANIC LETTERS
- Volume
- 11
- Number
- 1
- Start Page
- 17
- End Page
- 20
- ISSN
- 1523-7060
- Abstract
- We developed a novel regioselective synthesis of tetrasubstituted pyrroles via the classic 1,3-dipolar cycloaddition of alpha,beta-unsaturated benzofuran-3(2h)-one and azlactones (1) followed by spontaneous decarboxylation. The complete regiochemical control of tetrasubstituted pyrroles was confirmed by the orthogonal synthesis of complementary regioisomers (7a and 7b) simply by using different azlactones (1a and 1b, respectively).
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