Over 16% efficiency all-polymer solar cells by sequential deposition
DC Field | Value | Language |
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dc.contributor.author | Li, Bangbang | - |
dc.contributor.author | Zhang, Xuanyu | - |
dc.contributor.author | Wu, Ziang | - |
dc.contributor.author | Yang, Jie | - |
dc.contributor.author | Liu, Bin | - |
dc.contributor.author | Liao, Qiaogan | - |
dc.contributor.author | Wang, Junwei | - |
dc.contributor.author | Feng, Kui | - |
dc.contributor.author | Chen, Rui | - |
dc.contributor.author | Woo, Han Young | - |
dc.contributor.author | Ye, Fei | - |
dc.contributor.author | Niu, Li | - |
dc.contributor.author | Guo, Xugang | - |
dc.contributor.author | Sun, Huiliang | - |
dc.date.accessioned | 2022-06-22T08:41:27Z | - |
dc.date.available | 2022-06-22T08:41:27Z | - |
dc.date.created | 2022-06-22 | - |
dc.date.issued | 2022-06 | - |
dc.identifier.issn | 1674-7291 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/142242 | - |
dc.description.abstract | All-polymer solar cells (all-PSCs) have received extensive attention due to their excellent mechanical robustness and performance stability. However, the power conversion efficiency (PCE) of all-PSCs still lags behind those of organic solar cells (OSCs) based on non-fullerene small molecule acceptors. Herein, we report highly efficient all-PSCs via sequential deposition (SD) with donor and acceptor layers coated sequentially to optimize the film microstructure. Compared with the bulk heterojunction (BHJ) all-PSCs, an optimized morphology with vertical component distribution was achieved for the SD-processed all-PSCs due to the synergistic effect of swelling of polymer films and using additive. Such strategy involves using chlorobenzene as the first layer processing-solvent for polymer donor, chloroform as the second processing-solvent for polymer acceptor with trace 1-chlor-onaphthalene, efficiently promoting exciton dissociation and charge extraction and reducing trap-assisted recombination. Consequently, over 16% all-PSCs fabricated via SD method was realized for the first time, which is much higher than that (15.2%) of its BHJ counterpart and also among the highest PCEs in all-PSCs. We have further demonstrated the generality of this approach in various all-polymer systems. This work indicates that the SD method can yield excellent all-PSCs and provides a facile approach to fabricating high-performance all-PSCs. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | SCIENCE PRESS | - |
dc.title | Over 16% efficiency all-polymer solar cells by sequential deposition | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Woo, Han Young | - |
dc.identifier.doi | 10.1007/s11426-022-1247-1 | - |
dc.identifier.scopusid | 2-s2.0-85130929234 | - |
dc.identifier.wosid | 000795031100004 | - |
dc.identifier.bibliographicCitation | SCIENCE CHINA-CHEMISTRY, v.65, no.6, pp.1157 - 1163 | - |
dc.relation.isPartOf | SCIENCE CHINA-CHEMISTRY | - |
dc.citation.title | SCIENCE CHINA-CHEMISTRY | - |
dc.citation.volume | 65 | - |
dc.citation.number | 6 | - |
dc.citation.startPage | 1157 | - |
dc.citation.endPage | 1163 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Multidisciplinary | - |
dc.subject.keywordAuthor | all-polymer solar cells | - |
dc.subject.keywordAuthor | polymer acceptors | - |
dc.subject.keywordAuthor | planar heterojunction | - |
dc.subject.keywordAuthor | sequential deposition | - |
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