Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Yang, Xiao | - |
dc.contributor.author | Liu, Siyan | - |
dc.contributor.author | Liang, Tao | - |
dc.contributor.author | Yan, Xiulan | - |
dc.contributor.author | Zhang, Yunhui | - |
dc.contributor.author | Zhou, Yaoyu | - |
dc.contributor.author | Sarkar, Binoy | - |
dc.contributor.author | Ok, Yong Sik | - |
dc.date.accessioned | 2022-08-14T02:40:17Z | - |
dc.date.available | 2022-08-14T02:40:17Z | - |
dc.date.created | 2022-08-12 | - |
dc.date.issued | 2022-04-05 | - |
dc.identifier.issn | 0304-3894 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/143099 | - |
dc.description.abstract | Conventional adsorbents for decontaminating arsenic exhibit low efficacy for the removal of arsenite (As (III)). This study aims to develop a robust As adsorbent from natural magnetite (M-0) via a facile ball milling process, and evaluate their performance for decontaminating As(III) and As(V) in water and soil systems. The ball milling process decreased the particle size and crystallinity of M-0, resulting in pronounced As removal by the ball-milled magnetite (M-m). Ball milling under air facilitated the formation of Fe-OH and Fe-COOH functional groups on M-m interface, contributing to effective elimination of As(III) and As(V) via hydrogen bonding and complexation mechanisms. Synergistic oxidation effects of hydroxyl and carboxyl groups, and reactive oxygen species (O-2(-), and center dot OH) on the transformation of As(III) to As(V) during the adsorption were proposed to explain the enhanced As(III) removal by M-m. A short-term soil incubation experiment indicated that the addition of M-m (10 wt%) induced a decrease in the concentration of exchangeable As by 30.25%, and facilitated the transformation of water-soluble As into residual fraction. Ball milling thus is considered as an eco-friendly (chemical-free) and inexpensive (scalable, one-stage process) method for upgrading the performance of natural magnetite towards remediating As, particularly for tackling the highly mobile As(III). | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | ELSEVIER | - |
dc.subject | ZERO-VALENT IRON | - |
dc.subject | CONTAMINATED SOILS | - |
dc.subject | NANOPARTICLES | - |
dc.subject | WATER | - |
dc.subject | REMOVAL | - |
dc.subject | EQUILIBRIUM | - |
dc.subject | BIOCHAR | - |
dc.subject | OXIDES | - |
dc.subject | FE3O4 | - |
dc.subject | LEAD | - |
dc.title | Ball-milled magnetite for efficient arsenic decontamination: Insights into oxidation-adsorption mechanism | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Ok, Yong Sik | - |
dc.identifier.doi | 10.1016/j.jhazmat.2021.128117 | - |
dc.identifier.scopusid | 2-s2.0-85121919092 | - |
dc.identifier.wosid | 000752575300005 | - |
dc.identifier.bibliographicCitation | JOURNAL OF HAZARDOUS MATERIALS, v.427 | - |
dc.relation.isPartOf | JOURNAL OF HAZARDOUS MATERIALS | - |
dc.citation.title | JOURNAL OF HAZARDOUS MATERIALS | - |
dc.citation.volume | 427 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Engineering | - |
dc.relation.journalResearchArea | Environmental Sciences & Ecology | - |
dc.relation.journalWebOfScienceCategory | Engineering, Environmental | - |
dc.relation.journalWebOfScienceCategory | Environmental Sciences | - |
dc.subject.keywordPlus | ZERO-VALENT IRON | - |
dc.subject.keywordPlus | CONTAMINATED SOILS | - |
dc.subject.keywordPlus | NANOPARTICLES | - |
dc.subject.keywordPlus | WATER | - |
dc.subject.keywordPlus | REMOVAL | - |
dc.subject.keywordPlus | EQUILIBRIUM | - |
dc.subject.keywordPlus | BIOCHAR | - |
dc.subject.keywordPlus | OXIDES | - |
dc.subject.keywordPlus | FE3O4 | - |
dc.subject.keywordPlus | LEAD | - |
dc.subject.keywordAuthor | Arsenic | - |
dc.subject.keywordAuthor | Magnetite | - |
dc.subject.keywordAuthor | Ball milling | - |
dc.subject.keywordAuthor | Synergistic oxidation | - |
dc.subject.keywordAuthor | Sustainable environmental engineering | - |
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