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Electrochemical conversion of carbon dioxide over silver-based catalysts: Recent progress in cathode structure and interface engineering

Authors
Dang Le Tri NguyenDo, Ha HuuManh Tung NguyenVo, Dai-Viet N.Van-Huy NguyenChinh Chien NguyenKim, Soo YoungQuyet Van Le
Issue Date
28-4월-2021
Publisher
PERGAMON-ELSEVIER SCIENCE LTD
Keywords
CO2 electrochemical conversion; Ag-based catalysts; CO production; Electrode-electrolyte interface; Material engineering
Citation
CHEMICAL ENGINEERING SCIENCE, v.234
Indexed
SCIE
SCOPUS
Journal Title
CHEMICAL ENGINEERING SCIENCE
Volume
234
URI
https://scholar.korea.ac.kr/handle/2021.sw.korea/49414
DOI
10.1016/j.ces.2020.116403
ISSN
0009-2509
Abstract
Electrochemical CO2 reduction (ECR) to CO and other high-value chemicals is emerging as a prominent technology, which entails using the electricity produced from renewable energy resources to convert the problematic CO2 greenhouse gas into value-added chemicals and fuels. In addition to Au electrocatalysts, which are high-cost materials, Ag-based electrocatalysts have been regarded as promising ECR to CO alternatives in recent years, especially with their excellent activity and lowered cost of electrocatalyst synthesis because Ag is much more abundant and inexpensive. In this study, we firstly introduce some possible reaction mechanisms for Ag electrocatalysts in ECR to CO. To identify an outstanding strategy to develop a guideline for Ag-based electrocatalysts, we comprehensively reviewed recent advances in material development and interfacial engineering based on some critical factors and effects. Finally, a summary and prospects toward the future development of electrocatalysts for ECR are provided. (C) 2021 Elsevier Ltd. All rights reserved.
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