An Efficient Switching-Off of Coherent Anti-Stokes Raman Scattering via Double Stimulated Raman Scattering Processes of Heteromolecular Vibrational Modes
DC Field | Value | Language |
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dc.contributor.author | Lim, So Hee | - |
dc.contributor.author | Choi, Dae Sik | - |
dc.contributor.author | Rhee, Hanju | - |
dc.contributor.author | Cho, Minhaeng | - |
dc.date.accessioned | 2021-08-31T01:49:22Z | - |
dc.date.available | 2021-08-31T01:49:22Z | - |
dc.date.created | 2021-06-19 | - |
dc.date.issued | 2020-04-30 | - |
dc.identifier.issn | 1520-6106 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/56263 | - |
dc.description.abstract | Recently, we introduced a new switching-off technique applicable to subdiffraction-limited coherent Raman imaging, where a coherent anti-Stokes Raman scattering (CARS) signal can be selectively suppressed via competitive stimulated Raman scattering (SRS) processes between vibrational modes of a single molecular species. Here, we show that such a three-beam CARS suppression can be made via double SRS processes between vibrational modes of heteromolecular species, a mixture of paraffin oil and benzene. We achieve more than 80% suppression of the pump-Stokes-beam CARS signal for the ring-breathing mode (target mode) of benzene when the C-H stretching mode (acceptor mode) of paraffin oil is used to deplete the pump photons via the pump-depletion-beam SRS process. The freedom in the choice of acceptor mode for depletion, which could be a critical advantage of the present switching-off scheme, can be of use for overcoming current challenges of depletion-based super-resolution coherent Raman imaging of biomolecules. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.subject | STED MICROSCOPY REVEALS | - |
dc.subject | IN-VIVO | - |
dc.subject | DEPLETION | - |
dc.subject | RESOLUTION | - |
dc.subject | EMISSION | - |
dc.subject | BREAKING | - |
dc.subject | LIMIT | - |
dc.title | An Efficient Switching-Off of Coherent Anti-Stokes Raman Scattering via Double Stimulated Raman Scattering Processes of Heteromolecular Vibrational Modes | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Cho, Minhaeng | - |
dc.identifier.doi | 10.1021/acs.jpcb.0c03080 | - |
dc.identifier.scopusid | 2-s2.0-85084185970 | - |
dc.identifier.wosid | 000529877200015 | - |
dc.identifier.bibliographicCitation | JOURNAL OF PHYSICAL CHEMISTRY B, v.124, no.17, pp.3583 - 3590 | - |
dc.relation.isPartOf | JOURNAL OF PHYSICAL CHEMISTRY B | - |
dc.citation.title | JOURNAL OF PHYSICAL CHEMISTRY B | - |
dc.citation.volume | 124 | - |
dc.citation.number | 17 | - |
dc.citation.startPage | 3583 | - |
dc.citation.endPage | 3590 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.subject.keywordPlus | STED MICROSCOPY REVEALS | - |
dc.subject.keywordPlus | IN-VIVO | - |
dc.subject.keywordPlus | DEPLETION | - |
dc.subject.keywordPlus | RESOLUTION | - |
dc.subject.keywordPlus | EMISSION | - |
dc.subject.keywordPlus | BREAKING | - |
dc.subject.keywordPlus | LIMIT | - |
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