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Investigation of all-solid-state electrochromic devices with durability enhanced tungsten-doped nickel oxide as a counter electrode

Authors
Lee, Sang JinLee, Tae-GonNahm, SahnKim, Dong HunYang, Dae JinHan, Seung Ho
Issue Date
30-1월-2020
Publisher
ELSEVIER SCIENCE SA
Keywords
Electrochromic device; Tungsten-doped nickel oxide; Counter electrode; Flexible smart window
Citation
JOURNAL OF ALLOYS AND COMPOUNDS, v.815
Indexed
SCIE
SCOPUS
Journal Title
JOURNAL OF ALLOYS AND COMPOUNDS
Volume
815
URI
https://scholar.korea.ac.kr/handle/2021.sw.korea/57933
DOI
10.1016/j.jallcom.2019.152399
ISSN
0925-8388
Abstract
Films of tungsten-doped nickel oxide, denoted Ni1-xWx oxide as counter electrode in electrochromic devices were deposited onto indium tin oxide coated glass substrates by reactive dc magnetron sputtering using tungsten-doped nickel alloy target. Electrochromic properties of Ni(x)Wi(1-x) oxides were evaluated in lithium perchlorate in propylene carbonate. Enhanced cycle stability with moderate optical modulation was obtained for Ni1-xWx oxide film with x = 0.024. Significant degradation in pure NiO film during extended electrochemical cycling caused by microstructural deep trap sites was minimized by W doping. The EC device fabricated with WO3 thin film and Ni1-xWx oxide thin film with x = 0.024 showed stable optical modulation of about 2% reduction from 100 to 1000 cycles. Flexible EC device was also fabricated with WO3 thin film and Ni1-xWx oxide thin film with x = 0.024 deposited on c-ITO/graphene/PET electrode and showed stable cycling performance with maintaining optical modulation of Delta T approximate to 40%. (C) 2019 Elsevier B.V. All rights reserved.
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