Theoretical insights into selective electrochemical conversion of carbon dioxide
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Lee, Chan Woo | - |
dc.contributor.author | Kim, Chanyeon | - |
dc.contributor.author | Min, Byoung Koun | - |
dc.date.accessioned | 2021-09-01T17:21:10Z | - |
dc.date.available | 2021-09-01T17:21:10Z | - |
dc.date.created | 2021-06-19 | - |
dc.date.issued | 2019-03-12 | - |
dc.identifier.issn | 2196-5404 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/66675 | - |
dc.description.abstract | Electrochemical conversion of CO2 and water to valuable chemicals and fuels is one of the promising alternatives to replace fossil fuel-based processes in realizing a carbon-neutral cycle. For practical application of such technologies, suppressing hydrogen evolution reaction and facilitating the activation of stable CO2 molecules still remain major challenges. Furthermore, high production selectivity toward high-value chemicals such as ethylene, ethanol, and even n-propanol is also not easy task to achieve. To settle these challenges, deeper understanding on underlying basis of reactions such as how intermediate binding affinities can be engineered at catalyst surfaces need to be discussed. In this review, we briefly outline recent strategies to modulate the binding energies of key intermediates for CO2 reduction reactions, based on theoretical insights from density functional theory calculation studies. In addition, important design principles of catalysts and electrolytes are also provided, which would contribute to the development of highly active catalysts for CO2 electroreduction. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | SPRINGEROPEN | - |
dc.subject | CO2 ELECTRO-REDUCTION | - |
dc.subject | SUBSURFACE OXYGEN | - |
dc.subject | OXIDATION-STATE | - |
dc.subject | FORMIC-ACID | - |
dc.subject | ELECTROREDUCTION | - |
dc.subject | CATALYST | - |
dc.subject | MORPHOLOGY | - |
dc.subject | STABILITY | - |
dc.subject | MONOXIDE | - |
dc.title | Theoretical insights into selective electrochemical conversion of carbon dioxide | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Min, Byoung Koun | - |
dc.identifier.doi | 10.1186/s40580-019-0177-2 | - |
dc.identifier.scopusid | 2-s2.0-85072086497 | - |
dc.identifier.wosid | 000461046600001 | - |
dc.identifier.bibliographicCitation | NANO CONVERGENCE, v.6 | - |
dc.relation.isPartOf | NANO CONVERGENCE | - |
dc.citation.title | NANO CONVERGENCE | - |
dc.citation.volume | 6 | - |
dc.type.rims | ART | - |
dc.type.docType | Review | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Science & Technology - Other Topics | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalResearchArea | Physics | - |
dc.relation.journalWebOfScienceCategory | Nanoscience & Nanotechnology | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.relation.journalWebOfScienceCategory | Physics, Applied | - |
dc.subject.keywordPlus | CO2 ELECTRO-REDUCTION | - |
dc.subject.keywordPlus | SUBSURFACE OXYGEN | - |
dc.subject.keywordPlus | OXIDATION-STATE | - |
dc.subject.keywordPlus | FORMIC-ACID | - |
dc.subject.keywordPlus | ELECTROREDUCTION | - |
dc.subject.keywordPlus | CATALYST | - |
dc.subject.keywordPlus | MORPHOLOGY | - |
dc.subject.keywordPlus | STABILITY | - |
dc.subject.keywordPlus | MONOXIDE | - |
dc.subject.keywordAuthor | Electrocatalysis | - |
dc.subject.keywordAuthor | CO2 reduction | - |
dc.subject.keywordAuthor | Intermediate binding energy | - |
dc.subject.keywordAuthor | Theoretical calculation | - |
Items in ScholarWorks are protected by copyright, with all rights reserved, unless otherwise indicated.
(02841) 서울특별시 성북구 안암로 14502-3290-1114
COPYRIGHT © 2021 Korea University. All Rights Reserved.
Certain data included herein are derived from the © Web of Science of Clarivate Analytics. All rights reserved.
You may not copy or re-distribute this material in whole or in part without the prior written consent of Clarivate Analytics.