Fast two-step deposition of perovskite via mediator extraction treatment for large-area, high-performance perovskite solar cells
DC Field | Value | Language |
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dc.contributor.author | Kim, Young Yun | - |
dc.contributor.author | Park, Eun Young | - |
dc.contributor.author | Yang, Tae-Youl | - |
dc.contributor.author | Noh, Jun Hong | - |
dc.contributor.author | Shin, Tae Joo | - |
dc.contributor.author | Jeon, Nam Joong | - |
dc.contributor.author | Seo, Jangwon | - |
dc.date.accessioned | 2021-09-02T08:59:38Z | - |
dc.date.available | 2021-09-02T08:59:38Z | - |
dc.date.created | 2021-06-16 | - |
dc.date.issued | 2018-07-14 | - |
dc.identifier.issn | 2050-7488 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/74348 | - |
dc.description.abstract | As the efficiency of perovskite solar cells (PSCs) reached more than 22%, the large-area fabrication of PSCs became another issue receiving growing attention. For large-area PSCs, more reproducibility is required to precisely control the crystallization behavior of perovskites. A two-step process has been preferred to apply large-area coatings of perovskite because of its better reproducibility, but the process has suffered from slow and incomplete conversion of PbI2 to perovskite. In this paper, we propose a fast, simple, two-step methodmediator extraction treatment (MET)for the preparation of a high-quality perovskite film. In MET, a pre-deposited PbI2-DMSO complex film is converted into a peculiar PbI2 film with a porous morphology and unusual crystallographic orientation via the removal of DMSO. PbI2 could be completely converted into MAPbI(3) by a fast reaction with MAI molecules. We demonstrate that this MET process in MAPbI(3)-based PSCs can achieve 18.8% of the maximum power conversion efficiency (PCE) using spin-coating, and 18.3% of the maximum PCE using slot-die coating with a uniform distribution in a 10 x10 cm(2) substrate at a laboratory scale. Moreover, over 18% of PCE could be achieved in only 100 s, and with room-temperature processing. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | ROYAL SOC CHEMISTRY | - |
dc.subject | HIGH-EFFICIENCY | - |
dc.subject | TRANSPORTING LAYER | - |
dc.subject | HALIDE PEROVSKITES | - |
dc.subject | BASE ADDUCT | - |
dc.subject | CRYSTALLIZATION | - |
dc.subject | FILMS | - |
dc.subject | NANOCRYSTALS | - |
dc.subject | CONVERSION | - |
dc.subject | STABILITY | - |
dc.subject | ROUTE | - |
dc.title | Fast two-step deposition of perovskite via mediator extraction treatment for large-area, high-performance perovskite solar cells | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Noh, Jun Hong | - |
dc.identifier.doi | 10.1039/c8ta02868k | - |
dc.identifier.scopusid | 2-s2.0-85049501327 | - |
dc.identifier.wosid | 000437469300027 | - |
dc.identifier.bibliographicCitation | JOURNAL OF MATERIALS CHEMISTRY A, v.6, no.26, pp.12447 - 12454 | - |
dc.relation.isPartOf | JOURNAL OF MATERIALS CHEMISTRY A | - |
dc.citation.title | JOURNAL OF MATERIALS CHEMISTRY A | - |
dc.citation.volume | 6 | - |
dc.citation.number | 26 | - |
dc.citation.startPage | 12447 | - |
dc.citation.endPage | 12454 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Chemistry | - |
dc.relation.journalResearchArea | Energy & Fuels | - |
dc.relation.journalResearchArea | Materials Science | - |
dc.relation.journalWebOfScienceCategory | Chemistry, Physical | - |
dc.relation.journalWebOfScienceCategory | Energy & Fuels | - |
dc.relation.journalWebOfScienceCategory | Materials Science, Multidisciplinary | - |
dc.subject.keywordPlus | HIGH-EFFICIENCY | - |
dc.subject.keywordPlus | TRANSPORTING LAYER | - |
dc.subject.keywordPlus | HALIDE PEROVSKITES | - |
dc.subject.keywordPlus | BASE ADDUCT | - |
dc.subject.keywordPlus | CRYSTALLIZATION | - |
dc.subject.keywordPlus | FILMS | - |
dc.subject.keywordPlus | NANOCRYSTALS | - |
dc.subject.keywordPlus | CONVERSION | - |
dc.subject.keywordPlus | STABILITY | - |
dc.subject.keywordPlus | ROUTE | - |
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