Dual-comb spectroscopy of molecular electronic transitions in condensed phases
DC Field | Value | Language |
---|---|---|
dc.contributor.author | Cho, Byungmoon | - |
dc.contributor.author | Yoon, Tai Hyun | - |
dc.contributor.author | Cho, Minhaeng | - |
dc.date.accessioned | 2021-09-02T13:44:54Z | - |
dc.date.available | 2021-09-02T13:44:54Z | - |
dc.date.created | 2021-06-16 | - |
dc.date.issued | 2018-03-16 | - |
dc.identifier.issn | 2469-9926 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/76712 | - |
dc.description.abstract | Dual-comb spectroscopy (DCS) utilizes two phase-locked optical frequency combs to allowscanless acquisition of spectra using only a single point detector. Although recent DCS measurements demonstrate rapid acquisition of absolutely calibrated spectral lines with unprecedented precision and accuracy, complex phase-locking schemes and multiple coherent averaging present significant challenges for widespread adoption of DCS. Here, we demonstrate Global Positioning System (GPS) disciplined DCS of a molecular electronic transition in solution at around 800 nm, where the absorption spectrum is recovered by using a single time-domain interferogram. We anticipate that this simplified dual-comb technique with absolute time interval measurement and ultrabroad bandwidth will allow adoption of DCS to tackle molecular dynamics investigation through its implementation in time-resolved nonlinear spectroscopic studies and coherent multidimensional spectroscopy of coupled chromophore systems. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | AMER PHYSICAL SOC | - |
dc.subject | MODE-LOCKED LASERS | - |
dc.subject | OPTICAL FREQUENCY-SYNTHESIS | - |
dc.subject | NOBEL LECTURE | - |
dc.title | Dual-comb spectroscopy of molecular electronic transitions in condensed phases | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Yoon, Tai Hyun | - |
dc.contributor.affiliatedAuthor | Cho, Minhaeng | - |
dc.identifier.doi | 10.1103/PhysRevA.97.033831 | - |
dc.identifier.scopusid | 2-s2.0-85043981310 | - |
dc.identifier.wosid | 000427632500020 | - |
dc.identifier.bibliographicCitation | PHYSICAL REVIEW A, v.97, no.3 | - |
dc.relation.isPartOf | PHYSICAL REVIEW A | - |
dc.citation.title | PHYSICAL REVIEW A | - |
dc.citation.volume | 97 | - |
dc.citation.number | 3 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Optics | - |
dc.relation.journalResearchArea | Physics | - |
dc.relation.journalWebOfScienceCategory | Optics | - |
dc.relation.journalWebOfScienceCategory | Physics, Atomic, Molecular & Chemical | - |
dc.subject.keywordPlus | MODE-LOCKED LASERS | - |
dc.subject.keywordPlus | OPTICAL FREQUENCY-SYNTHESIS | - |
dc.subject.keywordPlus | NOBEL LECTURE | - |
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