Electrosprayed BiVO4 nanopillars coated with atomic-layer-deposited ZnO/TiO2 as highly efficient photoanodes for solar water splitting
DC Field | Value | Language |
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dc.contributor.author | Kim, Min-Woo | - |
dc.contributor.author | Kim, Karam | - |
dc.contributor.author | Ohm, Tae Yoon | - |
dc.contributor.author | Yoon, Hyun | - |
dc.contributor.author | Joshi, Bhavana | - |
dc.contributor.author | Samuel, Edmund | - |
dc.contributor.author | Swihart, Mark T. | - |
dc.contributor.author | Choi, Sung Kyu | - |
dc.contributor.author | Park, Hyunwoong | - |
dc.contributor.author | Yoon, Sam S. | - |
dc.date.accessioned | 2021-09-02T15:05:54Z | - |
dc.date.available | 2021-09-02T15:05:54Z | - |
dc.date.created | 2021-06-16 | - |
dc.date.issued | 2018-02-01 | - |
dc.identifier.issn | 1385-8947 | - |
dc.identifier.uri | https://scholar.korea.ac.kr/handle/2021.sw.korea/77402 | - |
dc.description.abstract | We report the fabrication and the performance in photoelectrochemical water splitting of thin films of electrostatically sprayed nanotextured bismuth vanadate (BiVO4) pillars coated with thin ZnO/TiO2 passivation layers formed by atomic layer deposition. The thin ZnO and TiO2 layers deposited on the BiVO4 nanopillars formed a heterostructure that promoted electron-hole separation and the migration of electrons toward the ITO substrate. The photocurrent density (PCD) of the ZnO/TiO2 coated BiVO4 was 2.5 times higher (2.25 mA/cm(2) at 1.2 V (versus Ag/AgCl)) than that of pristine BiVO4 (0.9 mA/cm(2) at 1.2 V (versus Ag/AgCl)). We present incident/absorbed photon-to-current efficiency and electrochemical impedance measurements confirming that this improvement is a result of the heterojunction produced by the conformal ZnO/TiO2 coating and discuss the mechanism of this dramatic enhancement of PCD. | - |
dc.language | English | - |
dc.language.iso | en | - |
dc.publisher | ELSEVIER SCIENCE SA | - |
dc.subject | CHARGE SEPARATION | - |
dc.subject | BISMUTH VANADATE | - |
dc.subject | PERFORMANCE | - |
dc.subject | TIO2 | - |
dc.subject | HETEROJUNCTION | - |
dc.subject | NANOCOMPOSITES | - |
dc.subject | PHOTOCATALYST | - |
dc.subject | NANOPARTICLES | - |
dc.subject | OXIDATION | - |
dc.subject | FILMS | - |
dc.title | Electrosprayed BiVO4 nanopillars coated with atomic-layer-deposited ZnO/TiO2 as highly efficient photoanodes for solar water splitting | - |
dc.type | Article | - |
dc.contributor.affiliatedAuthor | Yoon, Sam S. | - |
dc.identifier.doi | 10.1016/j.cej.2017.09.130 | - |
dc.identifier.scopusid | 2-s2.0-85033457569 | - |
dc.identifier.wosid | 000417304500075 | - |
dc.identifier.bibliographicCitation | CHEMICAL ENGINEERING JOURNAL, v.333, pp.721 - 729 | - |
dc.relation.isPartOf | CHEMICAL ENGINEERING JOURNAL | - |
dc.citation.title | CHEMICAL ENGINEERING JOURNAL | - |
dc.citation.volume | 333 | - |
dc.citation.startPage | 721 | - |
dc.citation.endPage | 729 | - |
dc.type.rims | ART | - |
dc.type.docType | Article | - |
dc.description.journalClass | 1 | - |
dc.description.journalRegisteredClass | scie | - |
dc.description.journalRegisteredClass | scopus | - |
dc.relation.journalResearchArea | Engineering | - |
dc.relation.journalWebOfScienceCategory | Engineering, Environmental | - |
dc.relation.journalWebOfScienceCategory | Engineering, Chemical | - |
dc.subject.keywordPlus | CHARGE SEPARATION | - |
dc.subject.keywordPlus | BISMUTH VANADATE | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | TIO2 | - |
dc.subject.keywordPlus | HETEROJUNCTION | - |
dc.subject.keywordPlus | NANOCOMPOSITES | - |
dc.subject.keywordPlus | PHOTOCATALYST | - |
dc.subject.keywordPlus | NANOPARTICLES | - |
dc.subject.keywordPlus | OXIDATION | - |
dc.subject.keywordPlus | FILMS | - |
dc.subject.keywordAuthor | Bismuth vanadate nanopillar | - |
dc.subject.keywordAuthor | Photoanode | - |
dc.subject.keywordAuthor | Water splitting | - |
dc.subject.keywordAuthor | Photocurrent density | - |
dc.subject.keywordAuthor | Atomic layer deposition | - |
dc.subject.keywordAuthor | Heterostructure | - |
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