Bentonite dispersions: Transition from liquid-like to solid-like behavior and cracking
- Authors
- Pelot, D. D.; Jun, S.; Yarin, A. L.
- Issue Date
- 5월-2015
- Publisher
- ELSEVIER
- Keywords
- Bentonite; Cracking; Yield stress; Bending; Buckling; Compression
- Citation
- JOURNAL OF NON-NEWTONIAN FLUID MECHANICS, v.219, pp.50 - 64
- Indexed
- SCIE
SCOPUS
- Journal Title
- JOURNAL OF NON-NEWTONIAN FLUID MECHANICS
- Volume
- 219
- Start Page
- 50
- End Page
- 64
- URI
- https://scholar.korea.ac.kr/handle/2021.sw.korea/93674
- DOI
- 10.1016/j.jnnfm.2015.03.001
- ISSN
- 0377-0257
- Abstract
- Cylindrical samples of 11-13 wt% aqueous bentonite dispersions with a range of resting times after preparation (0-72 h) were subject to axial squeezing and revealed a transition from a Bingham liquid-like behavior to solid-like behavior. The liquid-like behavior is characterized by viscous spreading arrested by the yield stress, whereas the solid-like behavior is characterized by stasis at lower loads followed by discontinuity of the displacement and cracking above some critical level of load. A mechanical response, dependent on resting time, implied irreversible aging as a result of slow swelling of the clay crystallites, i.e. the internal structure being built over time in the material at rest. Dispersions of 11 wt% and 12 wt% transitioned from liquid-like to solid-like behavior in a single experiment at a resting time of 24 h and 3 h, respectively. At higher concentrations (18-22 wt%) the material always behaves as a solid. The solid-like behavior is distinguished from the liquid-like behavior by the appearance of cracks. The additional bending and buckling experiments conducted with dispersions of 18-22 wt% revealed Young's moduli of 330-500 kPa, yield stresses of 9-15 kPa, cracking stresses of 15-25 kPa, and cracking strains of 8-10%. For all concentrations explored, a linear dependence of the yield stress on concentration was found. It is demonstrated for the first time using uniaxial compression that liquid bentonite dispersions at a concentration of 11-12 wt% reveal transition to a solid in a single experiment where they become capable of developing surfaces of discontinuity of the displacement. (C) 2015 Elsevier B.V. All rights reserved.
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