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Superprotonic Conductivity of a UiO-66 Framework Functionalized with Sulfonic Acid Groups by Facile Postsynthetic Oxidation

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dc.contributor.authorPhang, Won Ju-
dc.contributor.authorJo, Hyuna-
dc.contributor.authorLee, Woo Ram-
dc.contributor.authorSong, Jeong Hwa-
dc.contributor.authorYoo, Kicheon-
dc.contributor.authorKim, BongSoo-
dc.contributor.authorHong, Chang Seop-
dc.date.accessioned2021-09-04T17:05:21Z-
dc.date.available2021-09-04T17:05:21Z-
dc.date.created2021-06-18-
dc.date.issued2015-04-20-
dc.identifier.issn1433-7851-
dc.identifier.urihttps://scholar.korea.ac.kr/handle/2021.sw.korea/93823-
dc.description.abstractFacile postsynthetic oxidation of the thiol-laced UiO-66-type framework UiO-66(SH)(2) enabled the generation of UiO-66(SO3H)(2) with sulfonic acid groups covalently linked to the backbone of the system. The oxidized material exhibited a superprotonic conductivity of 8.4 x 10(-2) S cm(-1) at 80 degrees C and 90% relative humidity, and long-term stability of the conductivity was observed. This level of conductivity exceeds that of any proton-conducting MOF reported to date and is equivalent to the conductivity of the most effective known electrolyte, Nafion.-
dc.languageEnglish-
dc.language.isoen-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.subjectMETAL-ORGANIC FRAMEWORK-
dc.subjectHIGH PROTON CONDUCTIVITY-
dc.subjectFUEL-CELL APPLICATIONS-
dc.subjectPOROUS COORDINATION POLYMERS-
dc.subjectCARBON-DIOXIDE-
dc.subjectPORE SURFACE-
dc.subjectCONDUCTORS-
dc.subjectOPPORTUNITIES-
dc.subjectCATALYSIS-
dc.subjectTRANSPORT-
dc.titleSuperprotonic Conductivity of a UiO-66 Framework Functionalized with Sulfonic Acid Groups by Facile Postsynthetic Oxidation-
dc.typeArticle-
dc.contributor.affiliatedAuthorHong, Chang Seop-
dc.identifier.doi10.1002/anie.201411703-
dc.identifier.scopusid2-s2.0-84927722973-
dc.identifier.wosid000354190800028-
dc.identifier.bibliographicCitationANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.54, no.17, pp.5142 - 5146-
dc.relation.isPartOfANGEWANDTE CHEMIE-INTERNATIONAL EDITION-
dc.citation.titleANGEWANDTE CHEMIE-INTERNATIONAL EDITION-
dc.citation.volume54-
dc.citation.number17-
dc.citation.startPage5142-
dc.citation.endPage5146-
dc.type.rimsART-
dc.type.docTypeArticle-
dc.description.journalClass1-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.relation.journalResearchAreaChemistry-
dc.relation.journalWebOfScienceCategoryChemistry, Multidisciplinary-
dc.subject.keywordPlusMETAL-ORGANIC FRAMEWORK-
dc.subject.keywordPlusHIGH PROTON CONDUCTIVITY-
dc.subject.keywordPlusFUEL-CELL APPLICATIONS-
dc.subject.keywordPlusPOROUS COORDINATION POLYMERS-
dc.subject.keywordPlusCARBON-DIOXIDE-
dc.subject.keywordPlusPORE SURFACE-
dc.subject.keywordPlusCONDUCTORS-
dc.subject.keywordPlusOPPORTUNITIES-
dc.subject.keywordPlusCATALYSIS-
dc.subject.keywordPlusTRANSPORT-
dc.subject.keywordAuthormetal-organic frameworks-
dc.subject.keywordAuthorpostsynthetic oxidation-
dc.subject.keywordAuthorproton-conducting materials-
dc.subject.keywordAuthorsulfonic acid groups-
dc.subject.keywordAuthorthiol groups-
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