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초록
The quantum it of an excitonic wave and its coherent control in a nanochain with a nanoring are studied. The nanochain is comprised of six chlorophylls, where four chlorophylls compose the nanoring and two chlorophylls are attached at two opposite sites on the nanoring. The exciton dynamics and the correlation of the excitation between chlorophylls are analyzed for a. given configurational arrangement and dipolar orientation of the chlorophylls. The results of this study show that the excitation at specified chlorophylls is suppressed or enhanced by destructive Or constructive interference of the excitonic wave in the chlorophyll nanochain.
키워드
Chlorophyll nanochain; Chlorophyll nanoring; Resonant dipole-dipole interaction; Exciton dynamics; Exciton eigenstates; Interference of excitonic wave; RESONANCE ENERGY-TRANSFER; EXCITATION-ENERGY; COHERENCE; PHOTOSYNTHESIS; MEMBRANE; DYNAMICS; SYSTEMS; PROTEIN; ELECTRODYNAMICS; COMPLEXES
- 제목
- Control of Quantum Interference of an Excitonic Wave in a Chlorophyll Chain with a Chlorophyll Ring
- 저자
- Hong, Suc-Kyoung; Nam, Seog Woo; Yeon, Kyu Hwang
- 발행일
- 2010-07
- 유형
- Article
- 권
- 57
- 호
- 1
- 페이지
- 61 ~ 70