The emerging covalent organic frameworks (COFs) for solar-driven fuels production

  • Xia, C.
  • Kirlikovali, K.O.
  • Nguyen, T.H.C.
  • Nguyen, X.C.
  • Tran, Q.B.
  • ... Kim, S.Y.
  • 외 10명
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초록

Photocatalysis-driven fuel production has garnered increasing attention as it can potentially address current energy- and environmental-related issues of the 21st century. However, the current performance of materials used for this application is still limited due to poor light absorption, fast photogenerated electron-hole recombination, and inappropriate active sites. Covalent organic frameworks (COFs), which offer an excellent platform to construct unique photocatalytic systems, have emerged as potential materials for the production of solar fuels. In this review, we investigate the development of COFs for three primary solar-driven fuel production strategies: (i) hydrogen (H2) production, (ii) carbon dioxide (CO2) reduction, and (iii) dinitrogen (N2) fixation. This review provides a roadmap to design excellent COF-based photocatalysts and highlights current limitations in the field of photocatalysis. © 2021 Elsevier B.V.

키워드

Covalent organic frameworksFuel productionPhotocatalysisTRIAZINE-BASED FRAMEWORKSPHOTOCATALYTIC HYDROGEN-PRODUCTIONMETAL-FREECO2 REDUCTIONH-2 EVOLUTIONEFFICIENTNANOSHEETSSITESNANOPARTICLESCOCATALYST
제목
The emerging covalent organic frameworks (COFs) for solar-driven fuels production
저자
Xia, C.Kirlikovali, K.O.Nguyen, T.H.C.Nguyen, X.C.Tran, Q.B.Duong, M.K.Nguyen, Dinh M.T.Nguyen, D.L.T.Singh, P.Raizada, P.Nguyen, V.-H.Kim, S.Y.Singh, L.Nguyen, C.C.Shokouhimehr, M.Le, Q.V.
DOI
10.1016/j.ccr.2021.214117
발행일
2021-11-01
유형
Review
저널명
Coordination Chemistry Reviews
446