A Hydrogen-Bonded Organic Framework (HOF) with Type IV NH3 Adsorption Behavior

  • Kang, Dong Won
  • Kang, Minjung
  • Kim, Hyojin
  • Choe, Jong Hyeak
  • Kim, Dae Won
  • ... Hong, Chang Seop
  • 외 3명
Citations

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초록

An S-shaped gas isotherm pattern displays high working capacity in pressure-swing adsorption cycle, as established for CO2, CH4, acetylene, and CO. However, to our knowledge, this type of adsorption behavior has not been revealed for NH3 gas. Herein, we design and characterize a hydrogen-bonded organic framework (HOF) that can adsorb NH3 uniquely in an S-shape (type IV) fashion. While conventional porous materials, mostly with type I NH3 adsorption behavior, require relatively high regeneration temperature, this platform which has significant working capacity is easily regenerated and recyclable at room temperature.

키워드

ammonia adsorptionhydrogen-bonded organic frameworks (HOFs)porous materialsS-shaped isothermAMMONIA UPTAKEMECHANISMSTORAGEDESIGN
제목
A Hydrogen-Bonded Organic Framework (HOF) with Type IV NH3 Adsorption Behavior
저자
Kang, Dong WonKang, MinjungKim, HyojinChoe, Jong HyeakKim, Dae WonPark, Jeoung RyulLee, Woo RamMoon, DohyunHong, Chang Seop
DOI
10.1002/anie.201911087
발행일
2019-11-04
유형
Article
저널명
Angewandte Chemie International Edition
58
45
페이지
16152 ~ 16155