Giant Temperature Coefficient of Resistivity and Cryogenic Sensitivity in Silicon with Galvanically Displaced Gold Nanoparticles in Freeze-Out Region

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초록

The temperature coefficient of resistivity (TCR) and cryogenic sensitivity (Sr) of p-type silicon (p-Si) in the low-temperature region (10-30 K) are remarkably improved by increasing the coverage of galvanically displaced Au nanoparticles (NPs). By increase of the galvanic displacement time from 10 to 30 s, the average surface roughness (R-a) of the samples increases from 0.31 to 2.31 nm and the coverage rate of Au NPs increases from 3.1% to 21.9%. In the freeze-out region of the sample, an up to 103% increase of TCR and dramatically improved Sv of p-Si (similar to 5813%) are observed with Au coverage of 21.9% compared to p-Si without galvanically displaced Au NPs. By means of a finite element method (FEM) simulation study, it was found that the increase of surface roughness and a number of Au NPs on p-Si results in a higher temperature gradient and thermoelectric power to cause the unusual TCR and S-v values in the samples.

키워드

galvanic displacement; temperature coefficient of resistivity; bolometer; cryogenic sensitivity; Au nanoparticles; ELECTRICAL-PROPERTIES; THERMAL-CONDUCTIVITY; DOPED SILICON; AU DEPOSITION; AQUEOUS HF; BOLOMETER; SI(111); SENSORS; SURFACE; FILMS
제목
Giant Temperature Coefficient of Resistivity and Cryogenic Sensitivity in Silicon with Galvanically Displaced Gold Nanoparticles in Freeze-Out Region
저자
Lee, Seung-Hoon; Hwang, Seongpil; Jang, Jae-Won
DOI
10.1021/acsnano.6b07007
발행일
2017-02
유형
Article
저널명
ACS Nano
권
11
호
2
페이지
1572 ~ 1580