Heterogeneous selective oxidation of 5-hydroxymethyl-2-furfural (HMF) into 2,5-diformylfuran catalyzed by vanadium supported activated carbon in MIBK, extracting solvent for HMF

  • Antonyraj, Churchil A.
  • Kim, Bora
  • Kim, Yongjin
  • Shin, Seunghan
  • Lee, Kwan-Young
  • 외 2명
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초록

Heterogeneous selective oxidation of 5-hydroxymethyl-2-furfural (HMF) into 2,5-diformylfuran (DFF) using molecular oxygen and vanadium catalyst onto activated carbon in MIBK, extracting solvent for HMF, is described. Highly stable V2O5 supported on activated carbon catalyst was synthesized using V3+ (VCl3) precursor and confirmed by XPS analysis, which found to be highly active. A maximum HMF conversion of >95% with >96% DFF selectivity was achieved and this heterogeneous catalyst could be used 4 times without any significant loss of activity. (C) 2014 Elsevier B.V. All rights reserved.

키워드

5-Hydroxymethyl-2-furfural (HMF)2,5-Diformylfuran (DFF)OxidationVanadiumExtracting solventMethyl isobutyl ketone (MIBK)AEROBIC OXIDATIONONE-POTDERIVATIVESACIDCHEMICALSFUELS
제목
Heterogeneous selective oxidation of 5-hydroxymethyl-2-furfural (HMF) into 2,5-diformylfuran catalyzed by vanadium supported activated carbon in MIBK, extracting solvent for HMF
저자
Antonyraj, Churchil A.Kim, BoraKim, YongjinShin, SeunghanLee, Kwan-YoungKim, IlCho, Jin Ku
DOI
10.1016/j.catcom.2014.08.008
발행일
2014-12-05
유형
Article
저널명
Catalysis Communications
57
페이지
64 ~ 68