Dehydrogenation behavior of LiBH4/CaH2 composite with NbF5

  • Lim, Jae-Hag
  • Shim, Jae-Hyeok
  • Lee, Young-Su
  • Cho, Young Whan
  • Lee, Joonho
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초록

The dehydrogenation behavior of 6LiBH(4) + CaH2 + 0.2NbF(5) composite has been investigated. It is demonstrated that the addition of NbF5 is effective in lowering the dehydrogenation temperature of this composite. The composite starts dehydrogenation before the melting of LiBH4 and releases 9.1 wt.% hydrogen up to 400 degrees C. The equilibrium dehydrogenation temperature under I bar of hydrogen is estimated to be 309 degrees C with a reaction enthalpy change of 56.5kJ mol(-1) H-2, which is consistent with thermodynamic calculation. Crown Copyright (c) 2008 Published by Elsevier Ltd. on behalf of Acta Materialia Inc. All rights reserved.

키워드

Hydrogen storageHydridesMechanical millingThermodynamicsDifferential scanning calorimetryREVERSIBLE HYDROGEN STORAGESYSTEMSCA
제목
Dehydrogenation behavior of LiBH4/CaH2 composite with NbF5
저자
Lim, Jae-HagShim, Jae-HyeokLee, Young-SuCho, Young WhanLee, Joonho
DOI
10.1016/j.scriptamat.2008.08.037
발행일
2008-12
유형
Article
저널명
Scripta Materialia
59
12
페이지
1251 ~ 1254