1,3-Diketone-Mediated Synthesis of Symmetrical Aryl Imides from Activated Amides

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초록

Symmetrical aryl imides are synthesized from the reaction of activated amides such as N-phenyl-N-tosyl benzamides. The amine source is provided by lithium hexamethyldisilazide (LiHMDS), and a 1,3-diketone mediates the generation of the N-acyl donor from N,N-bis(trimethylsilyl)amide. Various symmetrical aryl amides are thus formed in moderate to good yields. The activated amide reacted with LiHMDS in the presence of 1,3-diketone to give the corresponding symmetrical aryl imides in good yields.+image

키워드

amideimidelithium hexamethyldisilane1,3-diketonetransamidationTRANSAMIDATIONAMINOCARBONYLATIONDERIVATIVESOXIDATIONACYLATIONN BOND-CLEAVAGECATALYZED ESTERIFICATIONSECONDARY AMIDESACID-CHLORIDESC CLEAVAGE
제목
1,3-Diketone-Mediated Synthesis of Symmetrical Aryl Imides from Activated Amides
저자
Park, Myeong SeongRajamanickam, Karthik RajanSong, Kwang HoLee, Sunwoo
DOI
10.1002/ajoc.202300469
발행일
2023-10-25
유형
Article; Early Access
저널명
Asian Journal of Organic Chemistry