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Reversible structural transformation and selective gas adsorption in a unique aqua-bridged Mn(II) metal-organic framework
- Authors
- Jeong, Euna; Lee, Woo Ram; Ryu, Dae Won; Kim, Yeonga; Phang, Won Ju; Koh, Eui Kwan; Hong, Chang Seop
- Issue Date
- 2013
- Publisher
- ROYAL SOC CHEMISTRY
- Citation
- CHEMICAL COMMUNICATIONS, v.49, no.23, pp.2329 - 2331
- Indexed
- SCIE
SCOPUS
- Journal Title
- CHEMICAL COMMUNICATIONS
- Volume
- 49
- Number
- 23
- Start Page
- 2329
- End Page
- 2331
- ISSN
- 1359-7345
- Abstract
- An aqua-bridged Mn metal-organic framework was prepared, and a dramatic structural transformation occurs upon solvent exchange-resolvation and desolvation-resolvation processes. The desolvated phase, formed by removing the aqua bridges, exhibits selective CO2 uptake over N-2, H-2, and CH4. Further, antiferromagnetic couplings are also found between Mn spins in the secondary building units.
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