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Palladium Catalysts for Dehydrogenation of Ammonia Borane with Preferential B-H Activation

Authors
Kim, Sung-KwanHan, Won-SikKim, Tae-JinKim, Tae-YoungNam, Suk WooMitoraj, MariuszPiekos, LukaszMichalak, ArturHwang, Son-JongKang, Sang Ook
Issue Date
28-7월-2010
Publisher
AMER CHEMICAL SOC
Citation
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.132, no.29, pp.9954 - 9955
Indexed
SCIE
SCOPUS
Journal Title
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume
132
Number
29
Start Page
9954
End Page
9955
URI
https://scholar.korea.ac.kr/handle/2021.sw.korea/116041
DOI
10.1021/ja101685u
ISSN
0002-7863
Abstract
Cationic Pd(II) complexes catalyzed the dehydrogenation of ammonia borane in the most efficient manner with the release of 2.0 equiv of H-2 in less than 60 s at 25 degrees C. Most of the hydrogen atoms were obtained from the boron atom of the ammonia borane. The first step of the dehydrogenation reaction was elaborated using density functional theory calculations.
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Graduate School > GREEN SCHOOL (Graduate School of Energy and Environment) > 1. Journal Articles
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