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Control of Quantum Interference of an Excitonic Wave in a Chlorophyll Chain with a Chlorophyll Ring

Authors
Hong, Suc-KyoungNam, Seog WooYeon, Kyu Hwang
Issue Date
7월-2010
Publisher
KOREAN PHYSICAL SOC
Keywords
Chlorophyll nanochain; Chlorophyll nanoring; Resonant dipole-dipole interaction; Exciton dynamics; Exciton eigenstates; Interference of excitonic wave
Citation
JOURNAL OF THE KOREAN PHYSICAL SOCIETY, v.57, no.1, pp.61 - 70
Indexed
SCIE
SCOPUS
KCI
Journal Title
JOURNAL OF THE KOREAN PHYSICAL SOCIETY
Volume
57
Number
1
Start Page
61
End Page
70
URI
https://scholar.korea.ac.kr/handle/2021.sw.korea/116095
DOI
10.3938/jkps.57.61
ISSN
0374-4884
Abstract
The quantum it of an excitonic wave and its coherent control in a nanochain with a nanoring are studied. The nanochain is comprised of six chlorophylls, where four chlorophylls compose the nanoring and two chlorophylls are attached at two opposite sites on the nanoring. The exciton dynamics and the correlation of the excitation between chlorophylls are analyzed for a. given configurational arrangement and dipolar orientation of the chlorophylls. The results of this study show that the excitation at specified chlorophylls is suppressed or enhanced by destructive Or constructive interference of the excitonic wave in the chlorophyll nanochain.
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