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Asymmetric Pauson-Khand-type reactions of 1,6-enynes using formaldehyde as a carbonyl source by cooperative dual rhodium catalysis
- Authors
- Furusawa, Takuma; Morimoto, Tsumoru; Ikeda, Keiichi; Tanimoto, Hiroki; Nishiyama, Yasuhiro; Kakiuchi, Kiyomi; Jeong, Nakcheol
- Issue Date
- 4-2월-2015
- Publisher
- PERGAMON-ELSEVIER SCIENCE LTD
- Keywords
- Asymmetric Pauson-Khand reaction; Decarbonylation; Formaldehyde; Enyne; Dual catalysis
- Citation
- TETRAHEDRON, v.71, no.5, pp.875 - 881
- Indexed
- SCIE
SCOPUS
- Journal Title
- TETRAHEDRON
- Volume
- 71
- Number
- 5
- Start Page
- 875
- End Page
- 881
- ISSN
- 0040-4020
- Abstract
- A dual neutral-cationic rhodium(I)-catalyzed Pauson-Khand-type reaction using formaldehyde as a carbonyl source is described. The simultaneous use of neutral rhodium(I) and cationic rhodium(l) complexes is required for efficient cooperative catalysis, which involves the neutral rhodium(l)-catalyzed decarbonylation of formaldehyde and the cationic rhodium(I)-catalyzed cyclocarbonylation of 1,6-enynes using the resulting carbonyl moiety. (C) 2014 Elsevier Ltd. All rights reserved.
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